浏览全部资源
扫码关注微信
Temporal and spatial distribution of ozone, meteorological effect and relation with its precursors in Guiyang city
- Acta Scientiarum Naturalium Universitatis Sunyatseni Vol. 59, Issue 5, Pages: 102-112(2020)
- 作者机构：
1.贵州财经大学地理环境与地球资源研究所，贵州 贵阳 550025
2.贵州财经大学管理科学与工程学院，贵州 贵阳 550025
3.贵州理工学院建筑与城市规划学院，贵州 贵阳 550003
- 作者简介：
- 基金信息：
DOI：10.13471/j.cnki.acta.snus.2020.02.21.2020D010
CLC： X515Published：25 September 2020，
Received：21 February 2020，
扫 描 看 全 文
苏志华,韩会庆,李莉等.贵阳市臭氧的时空分布、气象作用及其与前体物的关系[J].中山大学学报(自然科学版),2020,59(05):102-112.
SU Zhihua,HAN Huiqing,LI Li,et al.Temporal and spatial distribution of ozone, meteorological effect and relation with its precursors in Guiyang city[J].Acta Scientiarum Naturalium Universitatis Sunyatseni,2020,59(05):102-112.
苏志华,韩会庆,李莉等.贵阳市臭氧的时空分布、气象作用及其与前体物的关系[J].中山大学学报(自然科学版),2020,59(05):102-112. DOI： 10.13471/j.cnki.acta.snus.2020.02.21.2020D010.
SU Zhihua,HAN Huiqing,LI Li,et al.Temporal and spatial distribution of ozone, meteorological effect and relation with its precursors in Guiyang city[J].Acta Scientiarum Naturalium Universitatis Sunyatseni,2020,59(05):102-112. DOI： 10.13471/j.cnki.acta.snus.2020.02.21.2020D010.
摘要
利用贵阳市10个环境空气监测站发布的臭氧(O₃)及其前体物NO
2
和CO数据，结合同期的气象观测资料，研究2015年3月1日至2016年2月29日一个自然年O₃的时空分布特征、气象作用及其与前体物的关系。结果显示O
3
日变化显示出“单峰”型分布特征，一般在16：00~17：00点左右达到峰值。在3~10月与次年2月，O
3
月平均浓度整体较高，而11月、12月和次年1月，O
3
浓度整体偏低。O
3
-8h-max浓度与日照时数、日最高气温和风速呈正相关关系，与气压和相对湿度呈反相关关系；贵阳市O
3
浓度城区相对较低，郊区相对较高，从市中心到郊区污染逐渐增大。大气氧化剂O
X
的日变化特征呈“单峰”型分布，在春季和夏季的氧化性最强。O
X
在白天和夜晚的控制因素不同，O
X
在白天主要受O
3
控制，在夜间主要受NO
2
控制。
Abstract
Based on the continuous monitoring data of O
3
and its precursors NO
2
and CO from 10 air monitoring stations and meteorological observation data in the urban area of Guiyang during a natural year from March 1st
2015 to February 29th
2016
temporal and spatial distribution characteristics of O
3
meteorological effects and the relationship with its precursors were studied in Guiyang city. The results showed that the diurnal variation of O
3
showed a "single peak" distribution characteristic
which generally reaching its peak around 16：00 - 17：00. From March to October and in February of the next year
the monthly average O
3
concentration was relatively high
while in November
December and January of the next year
the O
3
concentration was relatively low. O
3
-8h-max concentration was positively correlated with sunshine hours
daily maximum temperature and wind speed
and negatively correlated with air pressure and average relative humidity. The O
3
concentration was relatively low in the urban area and relatively high in the suburbs
and the pollution gradually increased from the downtown to the suburbs. The diurnal variation of atmospheric oxidizer O
X
was characterized by "single peak" distribution
with the strongest oxidization in spring and summer. O
X
was controlled by different factors during the day and night. O
X
was mainly controlled by O
3
during the day and NO
2
during the night
respectively.
关键词
贵阳市臭氧（O3）气象作用前体物大气氧化剂（OX）
Keywords
Guiyangozone (O3)meteorological effectsprecursorsatmospheric oxidants (OX)
references
唐孝炎. 大气环境化学[M]. 北京: 高等教育出版社, 1990: 60-70.
TANG X Y. Atmospheric Environmental Chemistry[M]. Beijing: Higher Education Press, 1990: 60-70.
TU J, XIA Z G, WANG H S, et al. Temporal variations in surface ozone and its precursors and meteorological effects at an urban site in China[J]. Atmospheric Research, 2007, 85: 310-337.
MASCLIN S, FREY M M, ROGGE W F, et al. Atmospheric nitric oxide and ozone at the WAIS Divide deep coring site: a discussion of local sources and transport in West Antarctica[J]. Atmospheric Chemistry and Physics, 2013, 13: 8857-8877.
WANG Z S, LI Y T, CHEN T, et al. Ground-level ozone in urban Beijing over a 1-year period: Temporal variations and relationship to atmospheric oxidation[J]. Atmospheric Research, 2015, 164/165: 110-117.
VINGARZAN R. A review of surface ozone background levels and trends[J]. Atmospheric Environment, 2004, 38: 3431-3442.
ZHANG Q, YUAN B, SHAO M, et al. Variations of ground-level O3 and its precursors in Beijing in summertime between 2005 and 2011[J]. Atmospheric Chemistry and Physics, 2014, 14: 6089-6101.
舒卓智, 赵天良, 郑小波, 等. 清洁大气背景下贵阳空气质量变化及气象作用[J]. 中国环境科学, 2017, 37(12): 4460-4468.
SHU Z Z, ZHAO T L, ZHENG X B, et al. Air quality variations and meteorological drivers of Guiyang city in clean atmospheric environment[J]. China Environmental Science, 2017, 37(12): 4460-4468.
环境保护部. 环境空气质量标准（GB3095-2012）[S], 2012.
Ministry of Environmental Protection. Ambient air quality standards(GB 3095-2012) [S], 2012.
环境保护部. 环境空气质量指数(AQI) 技术规定（试行）[S], 2012.
Ministry of Environmental Protection. Technical regulation on ambient air quality index (AQI) (on trial) [S], 2012.
SINGLA V, SATSANGI A, PACHAURI T, et al. Ozone formation and destruction at a sub-urban site in North Central region of India[J]. Atmospheric Research, 2011, 101(1): 373-385.
PLOEGER F, FUEGLISTALER S, GROOB J U, et al. Insight from ozone and water vapour on transport in the tropical tropopause layer (TTL)[J]. Atmospheric Chemistry and Physics, 2011, 11(1): 407-419.
IM U, MARKAKIS K, POUPKOU A, et al. The impact of temperature changes on summer time ozone and its precursors in the Eastern Mediterranean[J]. Atmospheric Chemistry and Physics, 2011, 11(8)： 3847-3864.
WANG Y G，HOPKE P K，XIA X Y，et al． Source apportionment of airborne particulate matter using inorganic and organic species as tracers[J]. Atmospheric Environment, 2012, 55: 525-532．
GE B Z, XU X B, LIN W L, et al. Impact of the regional transport of urban Beijing pollutants on downwind areas in summer: ozone production efficiency analysis[J]. Tellus B: Chemical and Physical Meteorology, 2012, 64: 1-13.
CLEVELAND W S, GRAEDEL T E, KLEINER B, et al. Sunday and workday variations in photochemical air pollutants in New Jersey and New York[J]. Science,1974,186(4168): 1037-1038.
王占山, 李云婷, 陈添, 等. 北京市臭氧的时空分布特征[J]. 环境科学, 2014, 35(12): 4446-4453.
WANG Z S, LI Y T, CHEN T, et al. Temporal and spatial distribution characteristics of ozone in Beijing[J]. Environmental Science, 2014, 35(12): 4446-4453.
王占山, 李云婷, 陈添, 等. 北京城区臭氧日变化特征及与前体物的相关性分析[J]. 中国环境科学, 2014, 34(12): 3001-3008.
WANG Z S, LI Y T, CHEN T, et al. Analysis on diurnal variation characteristics of ozone and correlations with its precursors in urban atmosphere of Beijing[J]. China Environmental Science, 2014, 34(12): 3001-3008.
尚媛媛, 舒卓智, 郑小波, 等. 云贵高原城市冬夏季PM2.5与O3相互作用机理-以贵阳市为例[J]. 生态环境学报, 2018, 27(12): 2284-2289.
SHANG Y Y, SHU Z Z, ZHENG X B, et al. Interaction mechanism between PM2.5 and O3 in winter and summer in Yunnan-Guizhou plateau: a case study of Guiyang[J]. Ecology and Environmental Sciences, 2018, 27(12): 2284-2289.
ZHAO T, LIU D, ZHENG X, et al. Revealed variations of air quality in industrial development over a remote plateau of Southwest China: an application of atmospheric visibility data[J]. Meteorology and Atmospheric Physics, 2016, 129(6): 659-667.
李卫海, 李阳兵, 周焱, 等. 岩溶山地城市扩展空间差异的地形效应[J]. 地理科学进展, 2009, 28(1): 85-92.
LI W H, LI Y B, ZHOU Y, et al. The effect of karst mountain physiognomy on spatial process of urbanization in Guiyang city[J]. Progress in Geography, 2009, 28(1): 85-92
尚媛媛, 郑小波, 夏晓玲, 等. 贵阳市PM2.5分布特征及气象条件的影响[J]. 高原山地气象研究, 2018, 38(3): 45-50.
SHANG Y Y, ZHENG X B, XIA X L, et al. Characteristics of PM2.5 distribution and meteorological conditions in Guiyang[J]. Plateau and Mountain Meteorology Research, 2018, 38(3): 45-50.
HE Y Q, WANG Y J, KONG X G, et al. High resolution stalagmite δ18O records over the past 1 000 years from Dongge Cave in Guizhou[J]. Chinese Science Bulletin, 2005, 50(10):1003-1008.
董志南, 郑拴宁, 赵会兵, 等. 基于空间插值的风场模拟方法比较分析[J]. 地球信息科学学报, 2015, 17(1): 37-44.
DONG Z N, ZHENG S N, ZHAO H B, et al. Comparative analysis of methods of wind field simulation based on spatial interpolation[J]. Journal of Geo-information Sciences, 2015, 17(1): 37-44.
段平, 盛业华, 李佳, 等. 自适应的IDW插值方法及其在气温场中的应用[J]. 地理研究, 2014, 33(8): 1417-1426.
DUAN P, SHENG Y H, LI J, et al. Adaptive IDW interpolation method and its application in the temperature field[J]. Geographical Research, 2014, 33(8): 1417-1426.
李凯, 赵华甫, 吴克宁, 等. 土壤重金属Cd污染指数的适宜插值方法和合理采样数量研究[J]. 土壤通报, 2016, 47(5): 1056-1064.
LI K, ZHAO H F, WU K N, et al. Suitable interpolation method and reasonable sampling quantity of Cd pollution index in soil[J]. Chinese Journal of Soil Science, 2016, 47(5): 1056-1064.
徐家骝, 朱毓秀. 气象因子对近地面臭氧污染影响的研究[J]. 大气科学, 1994(6): 751-757.
XU J L, ZHU Y X. Effects of the meteorological factors on the ozone pollution near the ground[J]. Scientia Atmospherica Sinica, 1994（6）: 751-757.
包艳英, 徐洁, 张明明, 等.大连市臭氧污染特征及典型污染日成因[J]. 中国环境监测, 2017, 33(4): 167-178.
BAO Y Y, XU J, ZHANG M M, et al. The characteristics of ozone pollution and causes of a typical ozone pollution episode in Dalian [J]. Environmental Monitoring in China, 2017, 33(4): 167-178.
陈宜然, 陈长虹, 王红丽, 等. 上海臭氧及前体物变化特征与相关性研究[J]. 中国环境监测, 2011, 27(5): 44-49.
CHEN Y R, CHEN C H, WANG H L, et al. Analysis on concentration variety characteristics of ozone and correlations with its precursors in Shanghai [J]. Environmental Monitoring in China, 2011, 27(5): 44-49.
程念亮, 李云婷, 张大伟, 等. 2014年北京市城区臭氧超标日浓度特征及与气象条件的关系[J]. 环境科学, 2016, 37(6): 2041-1051.
CHENG N L, LI Y T, ZHANG D W, et al. Characteristics of ozone over standard and its relationships with meteorological conditions in Beijing city in 2014 [J]. Environmental Science, 2016, 37(6): 2041-1051.
安俊琳, 王跃思, 孙扬. 气象因素对北京臭氧的影响[J]. 生态环境学报, 2009, 18(3): 944-951.
AN J L, WANG Y S, SUN Y. Assessment of ozone variations and meteorological effects in Beijing [J]. Ecology and Environmental Sciences, 2009, 18(3): 944-951.
LAL S, NAJA M, SUBBARAYA B H. Seasonal variations in surface ozone and its precursors over an urban site in India[J]．Atmospheric Environment, 2000, 34(17): 2713-2724.
SILLMAN S, LOGAN J A, WOFSY S C. The sensitivity of ozone to nitrogen oxides and hydrocarbons in regional ozone episodes[J]. Journal of Geophysical Research Atmospheres, 1990, 95(D2): 1837-1851.
WANG Y S, YAO L, WANG L L, et al. Mechanism for the formation of the January 2013 heavy haze pollution episode over central and eastern China[J]. Science China(Earth Sciences), 2014, 57(1): 14-25.
LU K D, ROHRER F, HOLLAND F, et al. Observation and modelling of OH and HO2 concentrations in the Pearl River Delta 2006: a missing OH source in a VOC rich atmosphere[J]. Atmospheric Chemistry and Physics, 2012, 12: 1541-1569.
苏志华, 王建华. 贵阳市大气颗粒物的污染特征及其影响因素分析[J]. 中山大学学报(自然科学版), 2015, 54(5): 77-84.
SU Z H, WANG J H. Pollution characteristics and determinants of atmospheric particulate matter and its determinants in Guiyang [J]. Acta Scientiarum Naturalium University Sunyatseni, 2015, 54(5): 77-84.
CHEUNG V T F, WANG T. Observational study of ozone pollution at a rural site in the Yangtze Delta of China[J]. Atmospheric Environment, 2001, 35(29): 4947-4958.
STEPHENS S, MADRONICH S, WU F, et al. Weekly patterns of México City's surface concentrations of CO, NOX, PM10 and O3 during 1986-2007[J]. Atmospheric Chemistry and Physics, 2008, 8(17): 5313-5325.
SHAN W, YIN Y, ZHANG J, et al. Observational study of surface ozone at an urban site in East China[J]. Atmospheric Research, 2008, 89(3): 252-261.
0
Views
1
下载量
3
CSCD
- L-PDFDownload
- BibTeXDownload
- EndnoteDownload
- RefMan Download
- NoteExpressDownload
- NoteFirstDownload
Publicity Resources
Related Articles
Related Author
Related Institution
- Postal code：510275
- Tel：020-84112585，84113223 Email：xuebaozr@mail.sysu.edu.cn
- Technical support is provided by Beijing Founder electronics co., LTD 京ICP备09064830号-19
京公网安备11010802024621 - It is recommended to read the content of this site in Chrome&IE9+. Please switch to extreme mode in browser 360.
- Cookies We use cookies to help provide and enhance our service and tailor content. By continuing, you agree to the use of cookies.
